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entire vibrational spectrum of a sample in a single laser pulse, and with ultrafast time resolution. This spectroscopy is forbidden in isotropic bulk media (e.g., liquids, gases, and solids such as
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technologies, we will be able to interface with a broad range of AMO systems including individual, arrays, and ensembles of atoms and ions in free space as well dilute ensembles in solid state volumes
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or solid-state emitters with applications including sensing, time keeping, and quantum computing. Photonic metasurfaces [1,2] can be used as a platform for integrated fabrication of free-space optical
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